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The present Special Issue, dedicated to Professors Miguel Julve and Francisco (Paco) Lloret, two outstanding and pioneers scholars in the study of the magnetic properties of coordination compounds, gathers a good number of contributions from a large number of leading specialists in molecular magnetism of coordination compounds and metal-organic frameworks (MOFs). It comprises a laudation for Professors Miguel Julve and Paco Lloret, two review articles, and eighteen original research articles that pay tribute to their lives and works.