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Multifunctional polymer composites are a class of smart materials in which the polymer matrix is reinforced with fillers to tailor with different functionalities. The promise of integrating several functions into a single material is quite challenging. Moreover, their lightweight, durable, and customizable materials positions multifunctional polymer composites as a key enabler for next-generation technologies. This Reprint will focus on these aspects, thereby providing readers with an insightful idea of multifunctionality in polymer composites.