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This Reprint immerses the reader in cutting-edge research on enhancing the performance and sustainability of building materials. It explores innovative approaches in surface engineering and mechanical characterization, from evaluating the cracking resistance of in-service asphalt pavements and the durability of bridge deck systems to mitigating rebar corrosion in concrete. The studies within also unravel the potential of utilizing industrial by-products and eco-friendly composites, paving the way for a more circular economy in construction. Through insights from leading experts, this Collection embarks on a journey to unlock the full potential of advanced materials, seeking solutions that balance our infrastructural needs with the responsibility to build a more resilient and sustainable future.